Structure refinement and magnetic properties of synthetic Comml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" altimg="si128.svg" display="inline" id="d1e1336"mml:msubmml:mrow /mml:mrowmml:mn3/mml:mn/mml:mrow/mml:msub/mml:mathGemml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" altimg="si129.svg" display="inline" id="d1e1344"mml:msubmml:mrow /mml:mrowmml:mn2/mml:mn/mml:mrow/mml:msub/mml:mathOmml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" altimg="si130.svg" display="inline" id="d1e1352"mml:msubmml:mrow /mml:mrowmml:mn5/mml:mn/mml:mrow/mml:msub/mml:math(OH)mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" altimg="si131.svg" display="inline" id="d1e1361"mml:msubmml:mrow /mml:mrowmml:mn4/mml:mn/mml:mrow/mml:msub/mml:math phyllogermanate

Описание

Тип публикации: статья из журнала

Год издания: 2023

Идентификатор DOI: 10.1016/j.jmmm.2023.171262

Аннотация: Co3Ge2O5(OH)4 relates to a specific group of 1:1 layered compounds with an ability to form either platy or tubular particles depending on chemical composition. Despite successful synthesis and perspective application, there is a lack of information on its crystal structure and magnetic properties, granted by Co ions. Co3Ge2O5(OH)4 Показать полностьюphyllogermanate nanoparticles have been obtained using a hydrothermal method and characterised using powder X-ray diffraction and magnetisation measurements. Triclinic symmetry with a 1:P1 space group has been established. The unit cell contains three layers perpendicular to the c crystallographic direction, with 7.6 Å spacing and −b/3 shift of the middle layer. At a low magnetic field of 100 Oe the compound undergoes a magnetic transition at TN=5.2 K. The field of 9 T is not sufficient to take the sample to a magnetically saturated state with an asymptotic magnetic moment of 2.43 μB/Co2+. The estimations of the intralayer and interlayer exchange constants give values of J1/kB=2.75 K and J2/kB=0.25 K, respectively.

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Издание

Журнал: Journal of Magnetism and Magnetic Materials

Выпуск журнала: Т. 587

Номера страниц: 171262

ISSN журнала: 03048853

Издатель: Elsevier Science Publishing Company, Inc.

Персоны

  • Belskaya N.A. (Ioffe Institute, Polytechnicheskaya street, 26, St.-Petersburg, 194021, Russia)
  • Khrapova E.K. (Ioffe Institute, Polytechnicheskaya street, 26, St.-Petersburg, 194021, Russia)
  • Ivanova A.A. (Ioffe Institute, Polytechnicheskaya street, 26, St.-Petersburg, 194021, Russia)
  • Eremin E.V. (Reshetnev Siberian State University of Science and Technology, 31, Krasnoyarsky Rabochy Av., Krasnoyarsk, 660037, Russia)
  • Pavlov S.I. (Ioffe Institute, Polytechnicheskaya street, 26, St.-Petersburg, 194021, Russia)
  • Krasilin A.A. (Ioffe Institute, Polytechnicheskaya street, 26, St.-Petersburg, 194021, Russia)

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